A single mathematical law—Darcy’s law for shear-induced dispersion—could predict how fluids mix when they have different densities, viscosities, or temperatures, whether in a hydrogen micro-engine or an ocean current. The problem is that existing mixing theories break down when fluid properties vary. In hydrogen combustion, for example, the flame’s heat changes the gas density and viscosity, creating instabilities that current models cannot capture. This project aims to generalise a theory the researchers have already developed for combustion, extending it to any fluid system where shear forces drive mixing. They will test it on four classic problems: flame instabilities in thin cells, buoyancy-driven convection, double-diffusive convection, and surface-tension-driven flows. If successful, the work will give engineers a reliable tool to design hydrogen-powered micro-engines for drones and satellites, helping the UK move toward net-zero emissions. It will also provide oceanographers and physiologists with a unified framework for mixing in stratified fluids or biological flows. This is fundamental science—it builds the mathematical scaffolding for future applied research, much as earlier work on Taylor dispersion now underpins chromatography and drug delivery.
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The proposed work is an original research project with two main objectives: (1) to provide a generalised mixing theory for shear-induced dispersion and (2) to test the theory by applying it to four iconic mixing problems. The theory is pertinent to many engineering and real-life situations involving transport phenomena with variable density, viscosity, and other transport properties. Such situations are encountered in a variety of contexts with vastly different length scales—from the oceanic to the microscopic. The project is an ambitious attempt to generalise theoretical concepts and tools recently developed in our combustion-focused investigations in order to develop a theoretical framework with broad interdisciplinary applications. The theory will be applied to the following four problems: Flame instabilities in a Hele-Shaw cell, focusing on the coupling between Taylor dispersion and classical instabilities associated with variable properties, including the Darrieus–Landau instability (associated with variable density), the Saffman–Taylor instability (associated with variable viscosity), and the diffusive-thermal instability (associated with unequal mass and heat diffusivities). In the project, specific emphasis will be dedicated to hydrogen combustion. Effect of Taylor dispersion on the Rayleigh–Benard instability (associated with buoyancy) in a Hele-Shaw cell. Effect of Taylor dispersion on the double-diffusive convection instability (associated with buoyancy and differential diffusion) in a Hele-Shaw cell. Effect of Taylor dispersion on the Marangoni convection (associated with variable interfacial surface tension) in a thin fluid layer. The objectives of the work will be accomplished through a two-phase approach, the first being based on theoretical tools such as scaling analyses and perturbation methods and the second relying both on theoretical tools such as modelling and linear stability analyses and numerical tools involving numerical computations applied to the four selected problems. The success of the project will pave the way for future proposals that will benefit various beneficiaries. Such beneficiaries include applied mathematicians, fluid dynamicists, combustion scientists, oceanographers, physiologists, and others. A concrete illustration of research areas on which the project is expected to have an impact is that of hydrogen combustion, to which one of the test problems in this proposal is dedicated. Specifically, the outcomes of this problem should contribute to improving our understanding of hydrogen-flame dynamics in micro-engines that can power devices such as micro air vehicles (MAVs) and micro-satellites, thereby assisting engineers to design these devices more efficiently. With hydrogen being regarded as one of the most promising fuels for the future in order to decarbonise current fuels, this research should contribute to placing the UK at the forefront of international research efforts to address global greenhouse gas concerns. This is also in line with the EPSRC's strategic plan towards achieving "engineering net zero" via "transformative low and zero carbon—hydrogen and alternative liquid fuels".
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